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Abstract
Specific activities of natural (
238
U,
232
Th,
226
Ra and
40
K) and anthropogenic radionuclides (
137
Cs) in 160
soil samples collected from 16 districts of Songkhla province, have been measured and evaluated. Experimental
results were obtained by using a high-purity germanium (HPGe) detector and gamma spectrometry analysis
system at Nuclear and Material Physics laboratory in Department of Physics Faculty of Science Thaksin
University. Gamma ray radioactive standard sources Cesium-137 (Cs-137), Cobalt-60 (Co-60) and Barium-133
(
133
Ba) were used to calibrate the measurement system. The KCl and two
well-known reference materials (RGU-1
and RGTH-1) obtained from the International Atomic Energy Agency
were also used to analyze and compute the
40
K,
238
U (or
226
Ra) and
232
Th specific activity in all of the soil samples, respectively. The IAEA/SL-2 was also
used to evaluate the specific activity of
137
Cs in all soil samples. The measuring time of each sample is 10,800
seconds or 3 hours. It was found that, the soil specific activity ranges from 279.40 – 17523.33 Bq/kg for
40
K, 1.19
- 997.27 Bq/kg for
226
Ra, 3.84 – 192.98 Bq/kg for
232
Th and 0.00 – 24.58 Bq/kg for
137
Cs with mean values of
3149.26 ± 214.09 Bq/kg, 99.48 ± 6.64 Bq/kg, 54.19 ± 5.06 Bq/kg and 1.50 ± 0.76 Bq/kg, respectively. The
absorbed dose rates in air (D), the radium equivalent activity (Ra
eq
)
,
the external hazard index (H
ex
)
and
the annual
effective dose rate (ADE
out
)
due to
the calculated specific activities of
40
K,
226
Ra and
232
Th
were also evaluated and
ranges from 88.63 - 416.67 nGy/h,
177.77 - 807.51 Bq/kg, 0.48 – 2.18
and
0.11 - 0.51 mSv/y
with mean values of
210.00
nGy/h, 419.45 Bq/kg, 1.13 and 0.26
mSv/y, respectively
.
Moreover, all of these values were also compared
with nationally and internationally approved values.
Keywords
: Specific Activity, Soil, High-Purity Germanium (HPGe) Detector, Absorbed Dose Rate(D), Radium
Equivalent Activity(Ra
eq
), External Hazard Index(H
ex
), Annual Effective Dose Rate (ADE
out
)
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